Ab initio simulation of (Ba,Sr)TiO3 and (Ba,Ca)TiO3 perovskite solid solutions

Date
2019
Authors
Rusevich, Leonid L.
Zvejnieks, Guntars
Kotomin, Eugene A.
Journal Title
Journal ISSN
Volume Title
Publisher
Elsevier B.V.
Abstract
The results of ab initio (first-principles) computations of structural, elastic and piezoelectric properties of Ba(1−x)SrxTiO3 (BSTO) and Ba(1−x)CaxTiO3 (BCTO) perovskite solid solutions are presented, discussed and compared. Calculations are performed with the CRYSTAL14 computer code within the linear combination of atomic orbitals (LCAO) approximation, using advanced hybrid functionals of the density-functional-theory (DFT). Supercell model allows us to simulate solid solutions with different chemical compositions (x = 0, 0.125 and 0.25) within ferroelectric tetragonal phases (x < 0.3) of both solid solutions. It is shown that configurational disorder has to be taken into account in simulations of BCTO solid solutions, while for BSTO this effect is rather small. Both BSTO and BCTO show significantly enhanced piezoelectric properties, in a comparison with pure BaTiO3. However, these solid solutions demonstrate opposite behaviour of a tetragonal ratio c/a and elastic constants as the functions of chemical composition. It is predicted that due to decrease of the elastic constants in BCTO, it has much higher converse piezoelectric constants than BSTO.
Description
This research was supported by the ERA-NET HarvEnPiez project. Many thanks to R. Dovesi, M.M. Kržmanc and D. Gryaznov for fruitful discussions.
Keywords
Research Subject Categories::NATURAL SCIENCES:Physics , Perovskite solid solution , Lead-free piezoelectric , Ab initio , First-principles computation , Density functional theory (DFT)
Citation